posted on 2017-02-09, 02:00authored byAndrew Thomas Prata
This thesis presents
new and novel research on the satellite remote sensing of volcanic clouds,
which was motivated by the need to mitigate the associated impacts of volcanic
eruptions on civil aviation and provide deeper understanding on the radiative
effects of volcanic ash. Afternoon train (A-train) sensors were used to
characterise the horizontal and vertical evolution of the 2008 Chaitén
eruption from 2–10 May in southern Chile. The combination of the Atmospheric
InfraRed Sounder (AIRS) measurements with the Cloud-Aerosol Lidar with
Orthogonal Polarisation (CALIOP) is demonstrated to be an effective synergistic
technique capable of detecting volcanic ash in lidar backscatter returns.
Geometrically thin (< 400 m) and low-level (< 10 km) volcanic ash clouds
were identified. Ensemble forward trajectories from the Hybrid Single Particle
Lagrangian Integrated Trajectory (HYSPLIT) dispersion model were generated to
demonstrate how the new data could be used to improve Volcanic Ash Advisory
Centre (VAAC) operations.
The CALIOP/AIRS technique has also permitted identification
of stratospheric volcanic aerosols. The particulate lidar ratio (Sp) for two
classes of volcanic aerosols; fine ash and sulphate has been determined using
CALIOP observations. For the volcanic ash layers produced by the
Puyehue-Cordón Caulle eruption (June 2011) mean and median particulate lidar
ratios of 72 ± 15 sr and 69 sr, respectively, were obtained. For the Kasatochi
and Sarychev sulphates, mean (and standard deviation) of the retrieved lidar
ratios were 68 ± 21 sr (median 62 sr) and 68 ± 17 sr (median 62 sr),
respectively. The volume depolarisation ratio for fine ash was generally much
higher (δv up to 0.30) than that found for sulphates (δv from ∼0.05–0.10). However, the Sarychev observations
revealed an exponential decay in δv from 0.25 to 0.05. This finding highlights
the key importance of depolarisation measurements in understanding the compositional
evolution of volcanic aerosols. It is suggested that a criterion of δv < 0.2
could be used to discriminate between stratospheric ash and sulphate layers in
CALIOP observations.
Finally, A-train satellite measurements have been used to characterise
the immediate radiative effects of the Calbuco (April 2015) volcanic ash
clouds. The Calbuco ash layers were estimated to have produced a strong SW
cooling (−60 W/m-2) at the top of the atmosphere (TOA). However, this cooling
was offset by an even stronger LW warming (78 W/m-2), which resulted in an net
warming of ∼18 W/m-2 at TOA. In contrast, a net cooling (−58
W/m-2) was induced at the surface. The LW heating rates of the Calbuco ash
clouds were estimated to up to 20 K/day, while maximum SW heating was an order
of magnitude lower (∼3 K/day).